My favorite soundtracks on Neo-Geo games are:
Last Resort- "Jack To The Metro" (Stage 1) kicks ass.
Pulstar- All the tunes are great, though stage 2 is outstanding.
Viewpoint- Just jaw-dropping incredible. What more can I say?
KOF'94- Rugal's 2nd theme rocks. The Mexico, England, and USA BGMs also are great.
KOF'95- the Psycho Soldier team BGM and the one for King's team
Fatal Fury 3- Geese's new theme for this game.
KOF'96- King's BGM, Krauser's BGM, and Goenitz's BGM (this one is nice and ominous, fitting the wrecked stadium well)
KOF'97- Athena's theme, Billy Kane's theme.
KOF'98- All the tracks.
Neo Turf Masters- the Fujiyama Japan course BGM.
Bust-A-Move- OK, there's only one tune- but it is extremely good. Matter of fact, I just listened to it on Taito's Zuntata History Vol 2 CD.
Bust-A-Move Again EX- more tunes than the first one, and it's got a nice remix of the original.
Jackal
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